Efficient and highly enantioselective construction of trifluoromethylated quaternary stereogenic centers via high-pressure mediated organocatalytic conjugate addition of nitromethane to β, β-disubstituted enones.

DOI Number:

10.1021/ol502941d

Reaction Category:

RXNO ID:

RXNO_0000009

Educt:

beta,beta-disubstituted enones, nitromethane

Product:

1,3-disubstituted (R)-4,4,4-trifluoro-3-(nitromethyl)-butan-1-one

Catalyst:

N-[3,5-Bis(trifluoromethyl)phenyl]-N′-[(9R)-6′-methoxycinchonan-9-yl]thiourea

Cas No:

852913-25-8

Associated Product from Buchler GmbH:

N-[3,5-Bis(trifluoromethyl)phenyl]-N′-[(9R)-6′-methoxycinchonan-9-yl]thiourea

Cas No:

852913-25-8